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NZ732771B2 - Cgrp antagonist peptides - Google Patents
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NZ732771B2 - Cgrp antagonist peptides - Google Patents

Cgrp antagonist peptides Download PDF

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Publication number
NZ732771B2
NZ732771B2 NZ732771A NZ73277116A NZ732771B2 NZ 732771 B2 NZ732771 B2 NZ 732771B2 NZ 732771 A NZ732771 A NZ 732771A NZ 73277116 A NZ73277116 A NZ 73277116A NZ 732771 B2 NZ732771 B2 NZ 732771B2
Authority
NZ
New Zealand
Prior art keywords
cys
val
phe
3pal
gly
Prior art date
Application number
NZ732771A
Other versions
NZ732771A (en
Inventor
Guangcheng Jiang
Aleksandr K Rabinovich
Diaz Javier J Sueiras
Kazimierz Wisniewski
Original Assignee
Ferring Bv
Filing date
Publication date
Application filed by Ferring Bv filed Critical Ferring Bv
Priority claimed from PCT/EP2016/050110 external-priority patent/WO2016110499A1/en
Publication of NZ732771A publication Critical patent/NZ732771A/en
Publication of NZ732771B2 publication Critical patent/NZ732771B2/en

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Classifications

    • AHUMAN NECESSITIES
    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61KPREPARATIONS FOR MEDICAL, DENTAL OR TOILETRY PURPOSES
    • A61K38/00Medicinal preparations containing peptides
    • AHUMAN NECESSITIES
    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61PSPECIFIC THERAPEUTIC ACTIVITY OF CHEMICAL COMPOUNDS OR MEDICINAL PREPARATIONS
    • A61P25/00Drugs for disorders of the nervous system
    • A61P25/06Antimigraine agents
    • AHUMAN NECESSITIES
    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61PSPECIFIC THERAPEUTIC ACTIVITY OF CHEMICAL COMPOUNDS OR MEDICINAL PREPARATIONS
    • A61P43/00Drugs for specific purposes, not provided for in groups A61P1/00-A61P41/00
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D513/00Heterocyclic compounds containing in the condensed system at least one hetero ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for in groups C07D463/00, C07D477/00 or C07D499/00 - C07D507/00
    • C07D513/02Heterocyclic compounds containing in the condensed system at least one hetero ring having nitrogen and sulfur atoms as the only ring hetero atoms, not provided for in groups C07D463/00, C07D477/00 or C07D499/00 - C07D507/00 in which the condensed system contains two hetero rings
    • C07D513/04Ortho-condensed systems
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07KPEPTIDES
    • C07K7/00Peptides having 5 to 20 amino acids in a fully defined sequence; Derivatives thereof
    • C07K7/04Linear peptides containing only normal peptide links
    • C07K7/06Linear peptides containing only normal peptide links having 5 to 11 amino acids
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07KPEPTIDES
    • C07K7/00Peptides having 5 to 20 amino acids in a fully defined sequence; Derivatives thereof
    • C07K7/64Cyclic peptides containing only normal peptide links

Abstract

This disclosure relates to compounds of formula (I) or a pharmaceutically acceptable salt thereof: in which m, p, A, Ar1, Ar2, Ar3, R1, R2, and R3 are defined in the specification. The compounds of formula (I) can be used as CGRP antagonists and can be used to treat migraine.

Claims (17)

1. A compound of formula (I) or a pharmaceutically acceptable salt thereof: wherein 5 m is 0, 1, 2, 3, 4, or 5; p is 0, 1, 2, or 3;
2. A is single or double carbon-carbon bond; Ar1 is aryl or 5- or ered heteroaryl, each of which is optionally substituted with one or more substituents, each substituent independently being halogen, nitro, C1-C4 10 alkyl, C1-C4 hydroxyalkyl, ORa, or N(RaRa’), in which each Ra, independently, is H or C1- C4 alkyl and each Ra’, independently, is H or C1-C4 alkyl; Ar2 is aryl or 5- or 6-membered heteroaryl, each of which is optionally substituted with one or more substituents, each substituent independently being halogen, cyano, nitro, C1-C4 alkyl, C1-C4 aminoalkyl, C1-C4 yalkyl, ORb, ’), C(O)- 15 N(RbRb’), or NH-C(O)-N(RbRb’), in which each Rb, independently, is H or C1-C4 alkyl and each Rb’, ndently, is H or C1-C4 alkyl; Ar3 is aryl or 5- or 6-membered heteroaryl, each of which is optionally substituted with one or more substituents, each substituent independently being halogen, C1-C4 alkyl, C1-C4 hydroxyalkyl, ORc, or N(RcRc’), in which each Rc, independently, is H or C1-C4 20 alkyl and each Rc’, independently, is H or C1-C4 alkyl; each R1, independently, is C1-C4 alkyl, C1-C4 aminoalkyl, C1-C4 hydroxyalkyl, ORd, or C(O)-N(RdRd’), in which each Rd, independently, is H or C1-C4 alkyl and each Rd’, independently, is H or C1-C4 alkyl; R2 is -(CH2)n-R, in which n is 0, 1, 2, or 3 and R is N(CH3)2, NH(CH(CH3)2), NH- 5 H(NH2)-(CH2)4-N(CH3)2, NH-C(O)-CH2-(OCH2CH2)2-NH2, 3-amino-1,2,4- triazolyl, N(CH2CH3)2, or guanidino substituted with CH3; and each R3, ndently, is halogen, C1-C4 alkyl, or ORf, in which each Rf, independently, is H or C1-C4 alkyl. 10 2. The compound of claim 1, wherein Ar1 is phenyl, pyridinyl, oxazolyl, thiazolyl, olyl, pyrimidinyl, pyrolyl, or triazolyl, each of which is optionally substituted with one or more substituents, each substituent independently being F, Cl, NO2, CH3, CH2OH, or NH2. 15
3. The compound of claim 1, wherein Ar2 is phenyl or pyridinyl, each of which is optionally substituted with one or more substituents, each substituent independently being CH2NH2, C(O)NH2, OH, CN, CH2OH, NH2, or NH-C(O)-NH2.
4. The compound of claim 1, n Ar3 is pyridinyl.
5. The compound of claim 1, wherein m is 1.
6. The compound of claim 5, n R1 is OH, C(O)NH2, or CH2NH2. 25
7. The compound of claim 1, wherein n is 0, 1, or 2.
8. The compound of claim 1, wherein p is 0.
9. The compound of claim 1, wherein the compound is Oxazolecarbonyl- 30 D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Pro-Phe-Cys)-3Pal-NH2.
10. The compound of claim 1, wherein the compound is Picolinoyl-D-Val-Tyr-c(Cys-Dab(Et2)-Asp-Val-Gly-Pro-Phe-Cys)-3Pal-NH2; Picolinoyl-D-Val-Tyr-c(Cys-Dab(iPr)-Asp-Val-Gly-Pro-Phe-Cys)-3Pal-NH2; 5 noyl(5-F)-D-Val-Tyr-c(Cys-Orn(iPr)-Asp-Val-Gly-Pro-Phe-Cys)-3Pal-NH2; Picolinoyl-D-Val-Tyr-c(Cys-Orn(Et2)-Asp-Val-Gly-Pro-Phe-Cys)-3Pal-NH2; Picolinoyl(5-F)-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-3Pal-Cys)-3Pal- Picolinoyl(5-F)-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Pro-3Pal-Cys)-3Pal- 10 NH2; Oxazolecarbonyl-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Pro-3Pal-Cys)- 3Pal-NH2; Oxazolecarbonyl-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-Phe(3- )-Cys)-3Pal-NH2; 15 Oxazolecarbonyl-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-4Aph-Cys)- 3Pal-NH2; Oxazolecarbonyl-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-4Uph-Cys)- 3Pal-NH2; Picolinoyl(5-F)-D-Val-Tyr-c(Cys-Orn(iPr)-Asp-Val-Gly-Pro-Phe(4-CH2OH)-Cys)-3Pal- 20 NH2; Picolinoyl(3,5-F2)-D-Val-Tyr-c(Cys-Orn(iPr)-Asp-Val-Gly-Pro-Phe-Cys)-3Pal-NH2; Picolinoyl(5-F)-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-Phe(4-CH2OH)- Cys)-3Pal-NH2; Oxazolecarbonyl-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Pro-Phe(4- 25 CH2OH)-Cys)-3Pal-NH2; Oxazolecarbonyl-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-Phe(3-Cbm)- Cys)-3Pal-NH2; Picolinoyl(5-F)-D-Val-Phe(2-Cbm)-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-Phe(2-Cbm)- Cys)-3Pal-NH2; Oxazolecarbonyl-D-Val-Tyr-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-Phe(3-Cbm)-Cys)- 3Pal-NH2; Picolinoyl(5-F)-D-Val-Tyr-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-Phe(3-Cbm)-Cys)-3Pal- NH2; or 5 Picolinoyl-D-Val-Tyr-c(Cys-Orn(iPr)-Asp-Val-Gly-Dhp-Phe(4-CH2OH)-Cys)-3Pal-NH2.
11. A pharmaceutical ition, comprising the compound of any of claims 1-10 and a pharmaceutically acceptable carrier. 10
12. The pharmaceutical composition of claim 11, wherein the ition comprises an aqueous solution.
13. The pharmaceutical composition of claim 12, wherein the composition comprises a sodium chloride aqueous solution.
14. The pharmaceutical composition of claim 13, wherein the aqueous solution comprises about 0.9 wt% of sodium chloride.
15. A compound of any of claims 1 to 10 for, or for use in, the treatment of 20 migraine.
16. Use of a compound of any of claims 1 to 10 in the cture of a medicament for the treatment of migraine. 25
17. A nd selected from: Picolinoyl-D-Val-Tyr-c(Cys-Orn-Asp-Val-Gly-Pro-Phe(4-CH2OH)-Cys)-3Pal-NH2; or Picolinoyl(3,5-F2)-D-Val-Tyr-c(Cys-Arg-Asp-Val-Gly-Pro-Phe-Cys)-3Pal-NH2
NZ732771A 2016-01-06 Cgrp antagonist peptides NZ732771B2 (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US201562100371P 2015-01-06 2015-01-06
PCT/EP2016/050110 WO2016110499A1 (en) 2015-01-06 2016-01-06 Cgrp antagonist peptides

Publications (2)

Publication Number Publication Date
NZ732771A NZ732771A (en) 2024-07-05
NZ732771B2 true NZ732771B2 (en) 2024-10-08

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