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AU760014B2 - Utilization of a rubber-like polymer for producing roof sealing strips - Google Patents
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AU760014B2 - Utilization of a rubber-like polymer for producing roof sealing strips - Google Patents

Utilization of a rubber-like polymer for producing roof sealing strips Download PDF

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Publication number
AU760014B2
AU760014B2 AU14861/99A AU1486199A AU760014B2 AU 760014 B2 AU760014 B2 AU 760014B2 AU 14861/99 A AU14861/99 A AU 14861/99A AU 1486199 A AU1486199 A AU 1486199A AU 760014 B2 AU760014 B2 AU 760014B2
Authority
AU
Australia
Prior art keywords
roof sealing
sealing strips
rubber
polymer
weight
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
AU14861/99A
Other versions
AU1486199A (en
Inventor
Artur Peters
Udo Simonis
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Icopal Danmark ApS
Original Assignee
Henkel AG and Co KGaA
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Henkel AG and Co KGaA filed Critical Henkel AG and Co KGaA
Publication of AU1486199A publication Critical patent/AU1486199A/en
Application granted granted Critical
Publication of AU760014B2 publication Critical patent/AU760014B2/en
Assigned to Icopal Danmaerk a/s reassignment Icopal Danmaerk a/s Alteration of Name(s) in Register under S187 Assignors: HENKEL KOMMANDITGESELLSCHAFT AUF AKTIEN
Anticipated expiration legal-status Critical
Ceased legal-status Critical Current

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Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K5/00Use of organic ingredients
    • C08K5/04Oxygen-containing compounds
    • C08K5/10Esters; Ether-esters
    • C08K5/11Esters; Ether-esters of acyclic polycarboxylic acids
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F265/00Macromolecular compounds obtained by polymerising monomers on to polymers of unsaturated monocarboxylic acids or derivatives thereof as defined in group C08F20/00
    • C08F265/04Macromolecular compounds obtained by polymerising monomers on to polymers of unsaturated monocarboxylic acids or derivatives thereof as defined in group C08F20/00 on to polymers of esters
    • C08F265/06Polymerisation of acrylate or methacrylate esters on to polymers thereof
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L27/00Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Compositions of derivatives of such polymers
    • C08L27/02Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L27/04Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Compositions of derivatives of such polymers not modified by chemical after-treatment containing chlorine atoms
    • C08L27/06Homopolymers or copolymers of vinyl chloride
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L51/00Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers
    • C08L51/003Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers grafted on to macromolecular compounds obtained by reactions only involving unsaturated carbon-to-carbon bonds

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  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Compositions Of Macromolecular Compounds (AREA)
  • Sealing Material Composition (AREA)

Description

Utilization of a Rubber-Like Polymer for Producing Roof Sealing Strips Introduction This invention relates to the use of a rubber-like polymer for the production of roof sealing strips and to roof sealing strips containing this rubber-like polymer. This invention also relates to a method for producing roof sealing strips.
Prior Art Roof sealing strips are used in the building industry for sealing flat roofs and also at joins between individual structural elements. They are thus exposed to extreme weather conditions with the result that the materials used are expected to meet stringent requirements. They are required to be resistant to large variations in temperature and to moisture, UV radiation and strong winds or hail and snow. The roof sealing strips normally used are based on PVC and may contain an additional plasticizer and various stabilizers and fillers. Roof sealing strips known from the prior art are problematical in terms of their processability at low temperatures and particularly in terms of their weathering resistance.
The complex problem addressed by the invention was to develop roof sealing Sstrips from those known from the prior art which would have a distinctly higher weathering resistance and, at the same time, could be readily processed at various temperatures.
Description of the Invention Accordingly, in a first aspect, the present invention relates to the use in production of roof sealing strips of a rubber-like polymer consisting of the structural units butyl acrylate; at least one member from the group consisting of methyl methacrylate, ethyl 25 methacrylate, methyl acrylate and ethyl acrylate.
acrylonitrile, styrene, a semiester maleate soap and S: a crosslinking agent According to a second aspect of the present invention, there is provided A method for producing roof sealing strips comprising the steps of forming a roof sealing strip from a rubber-like polymer consisting of the structural units: butyl acrylate; at least one member selected from the group consisting of methyl methacrylate, ethyl methacrylate, methyl acrylate and ethyl acrylate; acrylonitrile; styrene; a semiester maleate soap; and l0 a crosslinking agent.
The invention also relates to a roof sealing strip produced by the method of the second aspect of the present invention.
It has now surprisingly been found that, by using the above-mentioned polymer in roof sealing strips, their weathering resistance can be distinctly improved and, at the same time, ready processability, particularly at low temperatures, is achieved. The roof sealing strips according to the invention have high elasticity and flexibility, even after prolonged weathering. At the same time, they are distinguished by their high chemical resistance, particularly to oils and solvents. Improved plasticizer retention has also been •observed so that the useful life of the roof sealing strips is distinctly increased.
Besides the rubber-like polymer, the roof sealing strips according to the invention preferably contain PVC although, basically, any materials known from the prior art for sealing strips are suitable plasticizers and stabilizers, fillers and other materials known from the prior art which are typically used in roof sealing strips.
Rubber-like polymer The rubber-like polymer to be used in accordance with the invention may be produced as described in EP 0 619 328. It is preferably composed of 40 to 80% by weight, preferably 50 to 80% by weight and more preferably 55 to 75% by weight butyl acrylate or optionally a mixture of butyl acrylate and 2-ethylhexyl acrylate containing up to 40% by weight of 2-ethylhexyl acrylate, 5 to 35% by weight and preferably 5 to 30 20% by weight of at least one substance selected from the group consisting of WO 00/24794 PCT/EP98/06705 methyl methacrylate, ethyl methacrylate, methyl acrylate or ethyl acrylate, 4 to 30% by weight, preferably 6 to 30% by weight and more preferably to 25% by weight acrylonitrile, 3 to 25% by weight, preferably 5 to 18% by weight and more preferably 8 to 14% by weight styrene, 0.5 to 8% by weight, preferably 1 to 5% by weight and more preferably 2 to 4% by weight of a maleate semiester soap and 0.25 to 8% by weight, preferably to 4% by weight and more preferably 1 to 3% by weight of a crosslinking agent.
A particularly preferred embodiment is characterized by the use of the rubber-like polymer marketed by Goodyear under the name of Sunigum®. The polymer is used in the roof sealing strips according to the invention in quantities of 1 to 30% by weight, preferably in quantities of 5 to by weight and more preferably in quantities of 8 to 15% by weight.
Polyvinyl chloride According to the invention, roof sealing strips of PVC with a PVC content of preferably 20 to 70% by weight and more particularly 30 to by weight are preferably used.
Plasticizers Any of the usual PVC-compatible plasticizers known from the prior art may be used as plasticizers. Typical plasticizers are, for example, derivatives of sylvinic acid or acetic acid derivatives, such as for example cumyl phenyl acetate, derivatives of adipic acid, such as benzyl octyl adipate, dibutyl adipate, diisobutyl adipate, di-(2-ethylhexyl)-adipate, diisononyl adipate, derivatives of azelaic acid, benzoic acid derivatives, polyphenyl derivatives, citric acid derivatives, epoxidized fatty derivatives, glycol derivatives and the other plasticizers mentioned on pages 5 and 6 of EP-B1 0 619 328.
Particularly preferred plasticizers are adipic acid polyesters, more WO 00/24794 PCT/EP98/06705 particularly in admixture with epoxidized triglycerides, preferably epoxidized soybean oil.
Plasticizers are normally present in the roof sealing strips in quantities of 15 to 65% by weight, preferably 20 to 45% by weight.
Stabilizers In order to increase their thermal stability, the roof sealing strips may additionally contain heat stabilizers known from the prior art, such as for example Pb stabilizers and/or Ba/Zn stabilizers, preferably Ca/Zn stabilizers. UV stabilizers, for example oxalanilides, amides, titanium dioxide, carbon black, more particularly Tinovin® and/or Chimasorp®, may also be present. Each stabilizer is present in a quantity of normally 0.01 to by weight and preferably 0.1 to 5% by weight. The total quantity of stabilizers normally does not exceed 20% by weight of the mixture.
Fillers The roof sealing strips may contain the usual fillers known from the prior art, for example chalk, talcum or silicas, although kaolin is particularly preferred as the filler. The quantity of fillers is 0.5 to 15% by weight and preferably 1 to 10% by weight.
The roof sealing strips may additionally contain other typical ingredients, such as for example lubricants, preferably Ca stearate, processing aids, gelling aids, UV converters and biocides, such as for example thiazoline derivatives, tributyl tin, chloroisothiazoline or oxy-bisphenoxyarsene, isothiazoline derivatives being particularly preferred.

Claims (8)

1. Use in production of roof sealing strips of a rubber-like polymer consisting of the structural units butyl acrylate; at least one member selected from the group consisting of methyl methacrylate, ethyl methacrylate, methyl acrylate and ethyl acrylate; acrylonitrile; styrene; a semiester maleate soap; and a crosslinking agent.
2. The use claimed in claim 1, wherein the roof sealing strips additionally contain polyvinyl chloride and a plasticizer.
3. The use claimed in claim 1 or 2, wherein the roof sealing strips additionally contain a UV stabilizer, a heat stabilizer and a filler.
4. Use of a rubber-like polymer substantially as hereinbefore described with reference to any one of the examples for the production of roof sealing strips.
A method for producing roof sealing strips comprising the steps of forming a roof sealing strip from a rubber-like polymer consisting of the structural units: butyl acrylate; at least one member selected from the group consisting of methyl methacrylate, ethyl methacrylate, methyl acrylate and ethyl acrylate; acrylonitrile; styrene; a semiester maleate soap; and a crosslinking agent.
6. A method for producing roof sealing strips comprising forming a roof sealing strip substantially as hereinbefore described with reference to any one of the examples.
7. Roof sealing strips produced by the method of claim 5 or 6. 0
8. Roof sealing strips according to claim 7, further comprising polyvinyl chloride, a plasticizer, a filler and stabilizers. Dated 24 February, 2003 Hen kel Kom manditgesellIschaft auf Aktien Patent Attorneys for the Applicant/Nominated Person SPRUSON FERGUSON 000 sees
AU14861/99A 1998-10-22 1998-10-22 Utilization of a rubber-like polymer for producing roof sealing strips Ceased AU760014B2 (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
PCT/EP1998/006705 WO2000024794A1 (en) 1998-10-22 1998-10-22 Utilization of a rubber-like polymer for producing roof sealing strips

Publications (2)

Publication Number Publication Date
AU1486199A AU1486199A (en) 2000-05-15
AU760014B2 true AU760014B2 (en) 2003-05-08

Family

ID=8167105

Family Applications (1)

Application Number Title Priority Date Filing Date
AU14861/99A Ceased AU760014B2 (en) 1998-10-22 1998-10-22 Utilization of a rubber-like polymer for producing roof sealing strips

Country Status (4)

Country Link
EP (1) EP1141055B1 (en)
AU (1) AU760014B2 (en)
DE (1) DE59812398D1 (en)
WO (1) WO2000024794A1 (en)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2007030151A1 (en) * 2005-09-02 2007-03-15 P & G Solutions, Inc. Weatherable corrosion-resistant flashing
CN101805478A (en) * 2010-05-11 2010-08-18 赵永生 Waterproof product containing ethylene-octylene copolymers and preparation method thereof

Families Citing this family (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN100441655C (en) * 2006-04-24 2008-12-10 何霖 Manufacturing Technology of Modified Polyvinyl Chloride Polymer Waterproof Membrane
DE102008024016A1 (en) * 2008-05-16 2009-11-19 Henkel Ag & Co. Kgaa Composition for producing a geomembrane
CN101805477B (en) * 2010-05-11 2012-05-09 赵根生 Waterproof product containing linear low density polyethylene and preparation method thereof
CN101831105B (en) * 2010-05-11 2012-07-18 冯青连 Ethylene-octene copolymer waterproof coil and preparation method thereof
CN108117704A (en) * 2016-11-28 2018-06-05 惠州市秋叶原实业有限公司 A kind of high-elastic Flame-Retardant and Oil-Resistant sizing materials of PVC

Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP0769507A2 (en) * 1995-10-20 1997-04-23 The Goodyear Tire & Rubber Company Rubbery polymer

Family Cites Families (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE4419007C2 (en) * 1994-05-31 2000-06-15 Freudenberg Carl Fa Process for the production of an impregnated flat gasket

Patent Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP0769507A2 (en) * 1995-10-20 1997-04-23 The Goodyear Tire & Rubber Company Rubbery polymer

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2007030151A1 (en) * 2005-09-02 2007-03-15 P & G Solutions, Inc. Weatherable corrosion-resistant flashing
CN101805478A (en) * 2010-05-11 2010-08-18 赵永生 Waterproof product containing ethylene-octylene copolymers and preparation method thereof

Also Published As

Publication number Publication date
EP1141055A1 (en) 2001-10-10
EP1141055B1 (en) 2004-12-15
AU1486199A (en) 2000-05-15
WO2000024794A1 (en) 2000-05-04
DE59812398D1 (en) 2005-01-20

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Free format text: IN VOL 14, NO 31, PAGE(S) 5604-5607 UNDER THE HEADING APPLICATIONS LAPSED, REFUSED OR WITHDRAWN PLEASE DELETE ALL REFERENCE TO APPLICATION NO. 14861/99 AND 14234/00

FGA Letters patent sealed or granted (standard patent)